Terahertz Fiber-Optic Lasers for Detection of Explosives
Terahertz-active gases inside hollow-core optical fibers would be optically pumped.
Fiber-optic lasers of a proposed type would serve as sources of coherent radiation at frequencies between 0.5 and 4.0 THz and output power levels ≥100 mW. In the original application envisioned in the proposal, these lasers would be parts of compact, man-portable instruments for detection of explosives.
The development of the proposed terahertz fiber-optic lasers would take advantage of, and extend, prior developments in the specialties of (1) generation of terahertz radiation by optical pumping of gases and (2) hollow-core photonic-crystal fibers.

- Optical pumping of gases has been used for several decades as a means of generating terahertz radiation. Efficient tabletop sources have been demonstrated and employed in many important applications. In a typical example of a source of this type, a midinfrared beam from a CO2 laser excites methanol molecules to a higher vibrational energy level, and terahertz photons are emitted in a radiative decay from the higher level to a lower level. At a pump power level of the order of 10 W, a source of this type is capable of producing tens of milliwatts of coherent terahertz optical power.
- Hollow-core photonic-crystal fibers have been fabricated from diverse materials, including plastics (see Figure 1). Hollow-core photonic-crystal fibers can be tailored to act as waveguides in selected frequency ranges.
A terahertz laser as proposed would include a plastic hollow-core photoniccrystal fiber tailored to support low-loss guiding of both a mid-infrared (e.g., CO2-laser) pump beam and the terahertz beam that one seeks to generate. The voids inside the hollow-core fiber would be filled with a suitable terahertzactive gas. The pump beam would be supplied by a sufficiently powerful gasmatched laser. If, for example, the terahertz- active filling gas were acetylene, a high-power, compact CO2 laser would be used as the pump.

The gas-filled hollow-core photoniccrystal fiber would be part of a terahertz optical resonator that would also include optical couplers and reflectors next to the input and output ends of the fiber (see Figure 2). An input mid-infrared coupler would enable efficient coupling of the pump beam into the fiber. An input terahertz reflector would be designed to be as highly reflective as possible at the intended terahertz operating frequency. An output terahertz coupler would be designed to optimize laser efficiency. To enhance the overall system efficiency, it may be desirable to design the resonator to provide for additional internal reflection of the pump beam at the input and output ends of the fiber.
Some of the risky and challenging aspects of the proposed development are the following:
- It is critical to design hollow-core photonic-crystal fibers to guide both mid-infrared pump and terahertz beams with losses low enough for efficient lasing. While guiding at single wavelengths has been demonstrated, simultaneous guiding at two wavelengths has not yet been realized.
- Filling the voids in hollow-core photonic-crystal fibers with suitable terahertz- active gases is a challenging task.
- Generation of terahertz beams in gasfilled photonic-crystal fibers has not been demonstrated yet.
- Engineering of coupling and reflective structures that provide for efficient and tailorable manipulation of two beams that differ greatly in wavelength is another challenging task.
This work was done by Antonije Radojevic of the C. S. Draper Laboratory, Inc. for the Naval Research Laboratory.
This Brief includes a Technical Support Package (TSP).

Terahertz Fiber-Optic Lasers for Detection of Explosives
(reference NRL-0023) is currently available for download from the TSP library.
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Overview
The document is a semi-annual status report on the "Terahertz Fiber Laser for Explosives Detection," submitted to the Department of the Navy's Office of Naval Research. The project, led by Dr. Antonije Radojevic at the C.S. Draper Laboratory, spans 24 months, starting from August 2006 to January 2007. The report covers the first six months of this effort.
The primary objective of the project is to develop a high-power (>100 mW), portable, coherent terahertz radiation source for explosives detection. This technology aims to surpass conventional methods, such as Schottky diodes and cryogenically cooled quantum cascade lasers, by providing improved sensitivity, selectivity, and a stand-off operating range greater than 20 meters, all within a compact, man-portable package.
During the initial phase, the research focused on modeling various types of photonic crystal fibers. Early analyses indicated potential in glass fibers; however, subsequent detailed modeling revealed unexpected material-related losses. Fortunately, the research pivoted towards hollow plastic fibers, which demonstrated significantly lower transmission losses in the terahertz regime. This shift is promising, as several research groups have successfully demonstrated terahertz waveguiding in hollow plastic optical fibers.
The report outlines the project's financial status, detailing expenditures, outstanding commitments, and the total grant value of $629,044. As of the report date, $299,684 has been funded, with a remaining balance of $329,360 to be funded. The financial summary indicates a careful allocation of resources, with a total expenditure of $71,835 and outstanding commitments of $34,600.
The document also notes a change in leadership, with Dr. Radojevic taking over as the Principal Investigator after the previous PI, Dr. Hakimi, left the laboratory. This transition had negligible impact on the project's timeline and objectives.
In summary, the report highlights the promising developments in terahertz fiber laser technology for explosives detection, emphasizing the shift to hollow plastic fibers as a viable solution. The project aims to create a new class of terahertz radiation sources that are efficient, portable, and effective for military applications, particularly in enhancing explosives detection capabilities.
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